TY - JOUR
T1 - Exploring Inverse Vulcanized Dicyclopentadiene As a Polymer Matrix for Carbon Fiber Composites
AU - Wickramasingha, Y. Athulya
AU - Stojcevski, Filip
AU - Eyckens, Daniel J.
AU - Hayne, David J.
AU - Chalker, Justin M.
AU - Henderson, Luke C.
PY - 2024/3
Y1 - 2024/3
N2 - Inverse vulcanization of waste or renewable dienes has generated materials with phenomenal properties across a spectrum of applications. Nevertheless, the use of these materials for structural applications remains a challenge. Here, the use of an inverse vulcanized cyclopentadiene polymer as a resin for carbon fiber reinforced composites is explored. The dynamic S─S bonds in the polymer matrix are used to repair composite specimens over 5 generations by heating the material to 140 °C. A range of composites are manufactured and evaluated for their flexural properties, using a range of fiber orientations. Finally, this polymer is used to reinforce a carbon fiber fabric composed entirely of reclaimed materials, constituting a composite entirely composed of waste materials and second life carbon fibers.
AB - Inverse vulcanization of waste or renewable dienes has generated materials with phenomenal properties across a spectrum of applications. Nevertheless, the use of these materials for structural applications remains a challenge. Here, the use of an inverse vulcanized cyclopentadiene polymer as a resin for carbon fiber reinforced composites is explored. The dynamic S─S bonds in the polymer matrix are used to repair composite specimens over 5 generations by heating the material to 140 °C. A range of composites are manufactured and evaluated for their flexural properties, using a range of fiber orientations. Finally, this polymer is used to reinforce a carbon fiber fabric composed entirely of reclaimed materials, constituting a composite entirely composed of waste materials and second life carbon fibers.
KW - carbon fiber
KW - interface
KW - inverse vulcanization
KW - repair
UR - http://www.scopus.com/inward/record.url?scp=85180699659&partnerID=8YFLogxK
UR - http://purl.org/au-research/grants/ARC/IH210100023
UR - http://purl.org/au-research/grants/ARC/DP180100094
UR - http://purl.org/au-research/grants/ARC/DP200100090
UR - http://purl.org/au-research/grants/ARC/DP230100587
UR - http://purl.org/au-research/grants/ARC/FT220100054
UR - http://purl.org/au-research/grants/ARC/IM230100048
U2 - 10.1002/mame.202300298
DO - 10.1002/mame.202300298
M3 - Article
AN - SCOPUS:85180699659
SN - 1438-7492
VL - 309
JO - Macromolecular Materials and Engineering
JF - Macromolecular Materials and Engineering
IS - 3
M1 - 2300298
ER -