Pulsed quantum cascade laser-based CRDS substance detection: real-time detection of TNT

C Harb, T Boyson, A Kallapur, I Petersen, M Calzada, T Spence, Kenneth Kirkbride, D Moore

    Research output: Contribution to journalArticlepeer-review

    23 Citations (Scopus)


    This paper presents experimental results from a pulsed quantum cascade laser based cavity ringdown spectrometer used as a high-Throughput detection system. The results were obtained from an optical cavity with 99.8% input and output coupling mirrors that was rapidly swept (0.2s to 7s sweep times) between 1582.25 cm-1 (6.3201μm) and 1697.00 cm-1 (5.8928μm ). The spectrometer was able to monitor gas species over the pressure range 585 torr to 1μtorr, and the analysis involves a new digital data processing system that optimises the processing speed and minimises the data storage requirements. In this approach we show that is it not necessary to make direct measurements of the ringdown time of the cavity to obtain the system dynamics. Furthermore, we show that correct data processing is crucial for the ultimate implementation of a wideband IR spectrometer that covers a range similar to that of commercial Fourier transform infrared instruments.

    Original languageEnglish
    Pages (from-to)15489-15502
    Number of pages14
    JournalOptics Express
    Issue number14
    Publication statusPublished - 2 Jul 2012


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